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- W3186843283 abstract "Abstract Two series of rod‐shaped dipolar organic compounds are synthesized, each of which contains an electron donor (D), an electron acceptor (A), and a rigid hydrocarbon spacer (S). The first series of S compounds belong to the derivatives of oligo‐norbornyl ( NB3 and NB4 ); and the second series of S the derivatives of a cage‐shaped heptacyclic tetradecane ( HT2a,b and HT4a,b ). The absorption/emission spectra and the oxidation/reduction potentials of D's and A's are measured, and the free energy of the photo‐excited electron transfer (PET) process is estimated according to the Marcus relationship. The degree of fluorescence quenching is found to be proportional to the corresponding free energy. The symmetry correlation between the frontier molecular orbitals of D and A is believed to play a significant role in the PET processes." @default.
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- W3186843283 date "2021-07-27" @default.
- W3186843283 modified "2023-10-18" @default.
- W3186843283 title "Synthesis of rod‐shaped dipolar compounds for the study of long‐range electronic interactions" @default.
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- W3186843283 doi "https://doi.org/10.1002/jccs.202100205" @default.
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