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• W3187061330 endingPage "113530" @default.
• W3187061330 startingPage "113530" @default.
• W3187061330 abstract "From the difficulty of awareness of abnormal concentrations of biochemical indexes in people's daily life come wearable sensing technologies. Recently, luminescent wearable biosensors are emerging with simple fabrication, easy use, cost-effectivity and reliability. But several challenges should be taken up, such as availability of varied analytes, high sensitivity, stability of enzymes, photostability, low signal noises and recyclability of sensors. Here, the Luminescent Wearable Sweat Tape (LWST) biosensor is developed via embedding multi-component nanoprobes onto microwell-patterned paper substrates of hollowed-out double-side tapes. The nanoprobes consist of responsive luminophores, enzyme-loaded gold nanocluster (AuNCs) nano-networks, which are wrapped by the switch, MnO 2 nanosheets. The responsive luminophores are constructed by 3 substitutable components: enzymes (uricase, GOx and alcohol dehydrogenase) for molecular target recognition, glutathione-protected AuNCs (yellow, red and green) for luminescent signal output and polycations PAH for integration. MnO 2 NSs as the switch can quench the emission of the AuNCs but degraded by the reductive product of incorporated enzymes. Thus, targeting analysts (uric acid, glucose and alcohol) can be dose-dependently detected through “turn-on” luminescence approach. After incorporating the nanoprobes into hollow-out tapes, the formed LWST biosensors can detect uric acid, glucose and alcohol in sweat with the help of a smartphone. Subsequently, we primarily apply them into human daily life scenario, sampling from dine parties, and the positive relationships of analyte intakes and the increase of analytes in sweat are significant with individual difference. • Sweat detection of uric acid, glucose and alcohol using luminescent wearable biosensors. • Open system for incorporation of various luminescent gold nanoclusters and enzymes. • Porous hydrogel structure enriching analytes and promote sensitivity of sensors. • Immobilization of enzymes improving their stability." @default.
• W3187061330 created "2021-08-02" @default.
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• W3187061330 date "2021-11-01" @default.
• W3187061330 modified "2023-10-17" @default.
• W3187061330 title "Luminescent wearable biosensors based on gold nanocluster networks for “turn-on” detection of Uric acid, glucose and alcohol in sweat" @default.
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• W3187061330 doi "https://doi.org/10.1016/j.bios.2021.113530" @default.
• W3187061330 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34325319" @default.
• W3187061330 hasPublicationYear "2021" @default.
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