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- W3187169635 abstract "Ammonia (NH3) plays an important role in agriculture and industry. The industry-scale production mainly depends on the Haber-Bosch process suffering from issues of environment pollution and energy consumption. Electrochemical reduction can degrade nitrite (NO2-) pollutants in the environment and convert it into more valuable NH3. Here, Ni2P nanosheet array on nickel foam is proposed as a 3D electrocatalyst for high-efficiency electrohydrogenation of NO2- to NH3 under ambient reaction conditions. When tested in 0.1 M phosphate buffer saline with 200 ppm NO2-, such Ni2P/NF is able to obtain a large NH3 yield rate of 2692.2 ± 92.1 μg h-1 cm-2 (3282.9 ± 112.3 μg h-1 mgcat.-1), a high Faradic efficiency of 90.2 ± 3.0%, and selectivity of 87.0 ± 1.7% at -0.3 V versus a reversible hydrogen electrode. After 10 h of electrocatalytic reduction, the conversion rate of NO2- achieves near 100%. The catalytic mechanism is further investigated by density functional theory calculations." @default.
- W3187169635 created "2021-08-16" @default.
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- W3187169635 date "2022-01-01" @default.
- W3187169635 modified "2023-10-15" @default.
- W3187169635 title "Ni2P nanosheet array for high-efficiency electrohydrogenation of nitrite to ammonia at ambient conditions" @default.
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- W3187169635 doi "https://doi.org/10.1016/j.jcis.2021.08.050" @default.
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