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- W3189381012 endingPage "113469" @default.
- W3189381012 startingPage "113469" @default.
- W3189381012 abstract "• In situ modified clay was examined for photocatalytic hydrogen evolution. • The incorporation of MoS x into Laponite D was realized for first time. • Photocatalytic activity of Lap/MoS x investigated by using three different sensitizers. Clay minerals have been proven as much attractive support materials for catalytic applications owing to its non-toxicity, low-cost, efficient surface area, ion exchange capacity and flat sheets. Laponite D is a layered silicate disc-type clay, which can provide efficient photocatalytic activity under visible light radiation due to its catalytic active surfaces and zwitterionic property. Herein, the photocatalytic studies based on the incorporation of MoS x onto Laponite D clay structure were carried out for the first time. Time dependent photocatalytic reactions were performed by using Laponite D, triethanolamine and eosin-Y dye as catalytically active surface, sacrificial electron donor and photosensitizer, respectively, in the absence and presence of ammonium tetrathiomolybdate as the precursor of in situ photodeposited MoS x co-catalyst. Laponite D/MoS x exhibited higher photocatalytic activity and stability than that of free-Laponite D and free-MoS x . Laponite D/MoS x enhanced the photocatalytic activity approximately 7- and 2-times compared to the free- Laponite D and free-MoS x , respectively. In addition, solar-to-hydrogen (STH) efficiencies are reached about 26% under solar irradiation for the Laponite D/MoS x in the presence of aqueous eosin-Y and triethanolamine media. Moreover, photocatalytic activities of eosin-Y sensitized Laponite D, free-MoS x and Laponite D/MoS x were compared to different xanthene type sensitizers." @default.
- W3189381012 created "2021-08-16" @default.
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- W3189381012 date "2021-10-01" @default.
- W3189381012 modified "2023-09-27" @default.
- W3189381012 title "In situ grown molybdenum sulfide on Laponite D clay: Visible-light-driven hydrogen evolution for high solar-to-hydrogen (STH) efficiencies" @default.
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- W3189381012 doi "https://doi.org/10.1016/j.jphotochem.2021.113469" @default.
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