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• W3189434410 endingPage "131541" @default.
• W3189434410 startingPage "131541" @default.
• W3189434410 abstract "Sulfate radical (SO4·-)-based AOPs has gradually become an attractive Fenton-like reaction protocol for refractory wastewater treatment. However, powder form of catalysts is not industrially favorable due to processing issues and challenges in transportation. Design efficient and stable modular catalysts is a promising alternative with application prospect. Here, a series of LDHs 3D porous foam as catalytic module with double metal-F interaction has been constructed by in-situ growth of CoFe-LDH nanoarrays on PVDF framework (CoFeLDH(F)/PVDF) through NH4F-assist hydrothermal, and used for activating PMS in water pollutant control. The high density CoFe-LDH nanoneedles and porous structure endow the catalytic foams with a number of accessible active sites, meanwhile the superhydrophilicity accelerates mass transfer. Moreover, metal-fluorine coordination can provide growth sites and modulate the charge distribution of metal ions, while metal-fluorine ionic bond makes more Co sites exposure. Consequently, the CoFeLDH(F)/PVDF foam displays ultrafast decolorization in flowing dye wastewater. A packed column module is also designed as proof-of-concept device for continuous degradation of simulated dyes polluted river water. This work provides a facile strategy for large-scale pre-treatment of high chroma wastewater in high-salinity, turbulent, and corrosive conditions." @default.
• W3189434410 created "2021-08-16" @default.
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• W3189434410 date "2021-12-01" @default.
• W3189434410 modified "2023-10-14" @default.
• W3189434410 title "LDHs-based 3D modular foam with double metal-fluorine interaction for efficiently promoting peroxymonosulfate activation in water pollutant control" @default.
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• W3189434410 doi "https://doi.org/10.1016/j.cej.2021.131541" @default.
• W3189434410 hasPublicationYear "2021" @default.
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