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• W3189509738 abstract "• The microstructure of the PPy aerogel could be tuned by precisely adjusting the molar ratio of methyl orange to pyrrole and the concentration of the pyrrole monomer. • A ultralong nanotubes aerogels with excellent structure-driven elasticity, adjustable flexibility, and high solar evaporation performance. • A salt-rejecting solar evaporator for long-term and stable evaporation under highly saline water. • Provides a strategy to design and develop new polymer-based nanotubular aerogels for efficient solar steam generation. Solar interface evaporation is considered to be a sustainable and environmentally friendly technology for obtaining fresh water from seawater. However, the preparation of photothermal conversion materials with excellent evaporation performance, good mechanical properties, and simple method for the solar interface evaporation still faces challenge. Herein, we report the fabrication of ultralong polypyrrole nanotubes aerogel-based solar steam generator through one-pot oxidative self-polymerization of pyrrole monomer using methyl orange as template and ferric chloride as oxidant. The as-prepared aerogel shows excellent elasticity, which can be compressed by 30% and recover to its original shape within a few seconds. In combination with abundant porosity (92.3%), low thermal conductivity (0.077 W m −1 K −1 ), super hydrophilic wettability and high light absorption (94%), the as-prepared aerogel shows a high solar-to-vapor efficiency above 74.5% even in high concentration saline (20%). This work provides new opportunities for effective design of conductive polymer-based photothermal monolithic materials with tunable porosity, adjustable morphology, required mechanical properties and high evaporation performance. Precisely controlled preparation of ultra-long polypyrrole nanotube aerogels for solar steam generation." @default.
• W3189509738 created "2021-08-16" @default.
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• W3189509738 date "2021-10-01" @default.
• W3189509738 modified "2023-09-30" @default.
• W3189509738 title "Ultralong polypyrrole nanotubes aerogels with excellent elasticity for efficient solar steam generation" @default.
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• W3189509738 doi "https://doi.org/10.1016/j.jtice.2021.07.043" @default.
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