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- W3189665096 abstract "We report a new synthetic methodology for polysulfonamides with well-defined linear and brush architectures by organocatalytic polymerizations. A new monomer, bis(2,3-disubstituted N-sulfonyl aziridine), has been rationally designed/synthesized and used in step-growth polymerization with various bisnucleophiles (dicarboxylic acids, diphenols, and dithiols). The branches or cross-linkages derived from the ring-opening polymerization of N-sulfonyl aziridines are suppressed using this specific bis(aziridine) monomer, resulting in a well-controlled linear polysulfonamide architecture. The synthesized polysulfonamides emit blue fluorescence in solution and exhibit excellent thermal properties with decomposition temperature at 5% weight loss (Td,5%) up to 360.0 °C and glass-transition temperature (Tg) ranging from 62.5 to 199.2 °C. Furthermore, a fast one-pot cascade approach has been developed toward polysulfonamide brush copolymers with a well-controlled grafted chain length." @default.
- W3189665096 created "2021-08-16" @default.
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- W3189665096 date "2021-08-11" @default.
- W3189665096 modified "2023-10-16" @default.
- W3189665096 title "Organocatalytic Synthesis of Polysulfonamides with Well-Defined Linear and Brush Architectures from a Designed/Synthesized Bis(<i>N</i>-sulfonyl aziridine)" @default.
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- W3189665096 doi "https://doi.org/10.1021/acs.macromol.1c01193" @default.
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