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- W3190029983 abstract "Abstract (HTz)[Ba(ClO 4 ) 3 ] (HTz=thiazolium cation, 1 ), a perchlorate‐based hybrid perovskite‐type single crystal undergoes sequential structural phase transitions at 143/154 K and 210/218 K. The perovskite‐type cage structure is composed of Ba 2+ nodes and ClO 4 − linkers to form anionic cage Ba 8 (ClO 4 ) 12 in which the HTz resides. It is notable that the anionic framework incorporating HTz is a perovskite‐type structure with the (4 12 ⋅ 6 3 ) framework. Various‐temperature single‐crystal structure analyses reveal the stepwise changed dynamics of HTz, and the distortion of the anionic cage Ba 8 (ClO 4 ) 12 are the origin of the phase transitions. We tend to attribute the switchable dielectric constant behavior mainly to order‐disorder transition of the HTzs and the rearrangement of the Ba 8 (ClO 4 ) 12 framework. Furthermore, dielectric switching is recorded. Our findings may prompt investigations of new perchlorate‐based organic‐inorganic hybrid perovskites." @default.
- W3190029983 created "2021-08-16" @default.
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- W3190029983 date "2021-08-31" @default.
- W3190029983 modified "2023-10-14" @default.
- W3190029983 title "High Quality of a Perchlorate‐Based Hybrid Perovskite‐Type Cage‐Like Single Crystal – Evidence of Temperature‐Induced Distinct Dielectric Transition" @default.
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- W3190029983 doi "https://doi.org/10.1002/ejic.202100624" @default.
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