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- W3190360070 abstract "Abstract The reaction of 1,3-bis(silyloxy)-1,3-butadienes with functionalized and nonfunctionalized acid chlorides and bis(acid chlorides) gives rise to the formation of a great variety of 1,3,5-tri- and 1,3,5,7-tetracarbonyl compounds and cyclic products derived from them. Examples include functionalized and nonfunctionalized 3,5-dioxopentanoates, 3,5-dioxopimelates, 3-alkylidene-3H-isobenzofuran-1-ones, salicylates, 3(2H)furanones, and 3-oxo-4-sulfonylesters. Methylation and cyclopropanation reactions of 1,3,5-tri- and 1,3,5,7-tetracarbonyl compounds do not provide access to the expected permethylated and cyclopropanated polycarbonyl compounds. However, the latter could be prepared by stepwise protocols. The reaction of 1,3,5-tri- and 1,3,5,7-tetracarbonyl compounds with dinucleophiles resulted in cyclization reactions to give a variety of heterocyclic structures. 1 Introduction 2 Reactions of 1,3-Bis(silyloxy)-1,3-butadienes with Acid Chlorides 3 Reactions of 1,3,5-Tri- and 1,3,5,7-Tetracarbonyl Compounds 4 Conclusion" @default.
- W3190360070 created "2021-08-16" @default.
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- W3190360070 date "2021-08-02" @default.
- W3190360070 modified "2023-09-27" @default.
- W3190360070 title "Synthesis and Reactions of 1,3,5-Tri- and 1,3,5,7-Tetracarbonyl Compounds" @default.
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- W3190360070 doi "https://doi.org/10.1055/s-0037-1610780" @default.
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