Matches in SemOpenAlex for { <https://semopenalex.org/work/W3190855211> ?p ?o ?g. }
- W3190855211 endingPage "2103857" @default.
- W3190855211 startingPage "2103857" @default.
- W3190855211 abstract "Oxygen reduction reaction (ORR) is an essential process for sustainable energy supply and sufficient chemical production in modern society. Single-atom catalysts (SACs) exhibit great potential on maximum atomic efficiency, high ORR activity, and stability, making them attractive candidates for pursuing next-generation catalysts. Despite substantial efforts being made on building diversiform single-atom active sites (SAASs), the performance of the obtained catalysts is still unsatisfactory. Fortunately, microenvironment regulation of SACs provides opportunities to improve activity and selectivity for ORR. In this review, first, ORR mechanism pathways on N-coordinated SAAS, electrochemical evaluation, and characterization of SAAS are displayed. In addition, recent developments in tuning microenvironment of SACs are systematically summarized, especially, strategies for microenvironment modulation are introduced in detail for boosting the intrinsic 4e−/2e− ORR activity and selectivity. Theoretical calculations and cutting-edge characterization techniques are united and discussed for fundamental understanding of the synthesis–construction–performance correlations. Furthermore, the techniques for building SAAS and tuning their microenvironment are comprehensively overviewed to acquire outstanding SACs. Lastly, by proposing perspectives for the remaining challenges of SACs and infant microenvironment engineering, the future directions of ORR SACs and other analogous procedures are pointed out." @default.
- W3190855211 created "2021-08-16" @default.
- W3190855211 creator A5026670698 @default.
- W3190855211 creator A5029425717 @default.
- W3190855211 creator A5031244158 @default.
- W3190855211 creator A5037878083 @default.
- W3190855211 creator A5041772520 @default.
- W3190855211 creator A5042351113 @default.
- W3190855211 creator A5079785501 @default.
- W3190855211 creator A5088447996 @default.
- W3190855211 date "2021-08-07" @default.
- W3190855211 modified "2023-10-17" @default.
- W3190855211 title "Recent Developments of Microenvironment Engineering of Single‐Atom Catalysts for Oxygen Reduction toward Desired Activity and Selectivity" @default.
- W3190855211 cites W1168565912 @default.
- W3190855211 cites W1537110470 @default.
- W3190855211 cites W1766028599 @default.
- W3190855211 cites W1979371521 @default.
- W3190855211 cites W1989715071 @default.
- W3190855211 cites W2012759651 @default.
- W3190855211 cites W2024805067 @default.
- W3190855211 cites W2034291571 @default.
- W3190855211 cites W2058965957 @default.
- W3190855211 cites W2095179527 @default.
- W3190855211 cites W2096065466 @default.
- W3190855211 cites W2099703449 @default.
- W3190855211 cites W2110534188 @default.
- W3190855211 cites W2123516051 @default.
- W3190855211 cites W2134716155 @default.
- W3190855211 cites W2154669151 @default.
- W3190855211 cites W2154763595 @default.
- W3190855211 cites W2181522365 @default.
- W3190855211 cites W2218721720 @default.
- W3190855211 cites W2299947148 @default.
- W3190855211 cites W2313881619 @default.
- W3190855211 cites W2346536990 @default.
- W3190855211 cites W2411120010 @default.
- W3190855211 cites W2520851868 @default.
- W3190855211 cites W2531551506 @default.
- W3190855211 cites W2536246483 @default.
- W3190855211 cites W2542984143 @default.
- W3190855211 cites W2550301288 @default.
- W3190855211 cites W2558739653 @default.
- W3190855211 cites W2558998316 @default.
- W3190855211 cites W2565767854 @default.
- W3190855211 cites W2591409535 @default.
- W3190855211 cites W2591446277 @default.
- W3190855211 cites W2592903883 @default.
- W3190855211 cites W2606430471 @default.
- W3190855211 cites W2607231338 @default.
- W3190855211 cites W2611902734 @default.
- W3190855211 cites W2612700249 @default.
- W3190855211 cites W2620858952 @default.
- W3190855211 cites W2624063830 @default.
- W3190855211 cites W2742325036 @default.
- W3190855211 cites W2745369682 @default.
- W3190855211 cites W2748096516 @default.
- W3190855211 cites W2754661150 @default.
- W3190855211 cites W2755768317 @default.
- W3190855211 cites W2766456865 @default.
- W3190855211 cites W2767545890 @default.
- W3190855211 cites W2767948854 @default.
- W3190855211 cites W2771332964 @default.
- W3190855211 cites W2774418387 @default.
- W3190855211 cites W2778748326 @default.
- W3190855211 cites W2784438572 @default.
- W3190855211 cites W2784943348 @default.
- W3190855211 cites W2785768358 @default.
- W3190855211 cites W2786858597 @default.
- W3190855211 cites W2790507915 @default.
- W3190855211 cites W2790537868 @default.
- W3190855211 cites W2790851364 @default.
- W3190855211 cites W2791305871 @default.
- W3190855211 cites W2792063676 @default.
- W3190855211 cites W2792542793 @default.
- W3190855211 cites W2794309598 @default.
- W3190855211 cites W2795293472 @default.
- W3190855211 cites W2795368538 @default.
- W3190855211 cites W2800356477 @default.
- W3190855211 cites W2800985602 @default.
- W3190855211 cites W2801659239 @default.
- W3190855211 cites W2801820474 @default.
- W3190855211 cites W2802378983 @default.
- W3190855211 cites W2802791016 @default.
- W3190855211 cites W2805483123 @default.
- W3190855211 cites W2805633012 @default.
- W3190855211 cites W2806308248 @default.
- W3190855211 cites W2806432392 @default.
- W3190855211 cites W2806882524 @default.
- W3190855211 cites W2808136178 @default.
- W3190855211 cites W2809416657 @default.
- W3190855211 cites W2810052757 @default.
- W3190855211 cites W2883112453 @default.
- W3190855211 cites W2883459753 @default.
- W3190855211 cites W2885206286 @default.
- W3190855211 cites W2885332738 @default.
- W3190855211 cites W2885750107 @default.
- W3190855211 cites W2888882000 @default.
- W3190855211 cites W2889270496 @default.