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- W3190991509 abstract "Translation of redox biocatalysis into a commercial hydrogenation flow reactor, with in-built electrolytic H 2 generation, was achieved using immobilized enzyme systems. Carbon-supported biocatalysts were first tested in batch mode, and were then transferred into continuous flow columns for H 2 -driven, NADH-dependent asymmetric ketone reductions. The biocatalysts were thus handled comparably to heterogeneous metal catalysts, but operated at room temperature and 1–50 bar H 2 , highlighting that biocatalytic strategies enable implementation of hydrogenation reactions under mild–moderate conditions. Continuous flow reactions were demonstrated as a strategy for process intensification; high conversions were achieved in short residence times, with a high biocatalyst turnover frequency and productivity. These results show the prospect of using enzymes in reactor infrastructure designed for conventional heterogeneous hydrogenations." @default.
- W3190991509 created "2021-08-16" @default.
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- W3190991509 date "2021-08-06" @default.
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- W3190991509 title "Boosting the Productivity of H2-Driven Biocatalysis in a Commercial Hydrogenation Flow Reactor Using H2 From Water Electrolysis" @default.
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- W3190991509 doi "https://doi.org/10.3389/fceng.2021.718257" @default.
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