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- W3191160956 abstract "A catalyst-controlled enantiodivergent bromolactonization of olefinic acids has been developed. Quinine-derived amino-amides bearing the same chiral core but different achiral aryl substituents were used as the catalysts. Switching the methoxy substituent in the aryl amide system from meta- to ortho-position results in a complete switch in asymmetric induction to afford the desired lactone in good enantioselectivity and yield. Mechanistic studies, including chemical experiments and density functional theory calculations, reveal that the differences in steric and electronic effects of the catalyst substituent alter the reaction mechanism." @default.
- W3191160956 created "2021-08-16" @default.
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- W3191160956 date "2021-08-05" @default.
- W3191160956 modified "2023-10-18" @default.
- W3191160956 title "A Catalyst-Controlled Enantiodivergent Bromolactonization" @default.
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- W3191160956 doi "https://doi.org/10.1021/jacs.1c05680" @default.
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