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- W3191729377 abstract "Abstract Photocatalytic hydrogen energy production through water splitting paves a promising pathway for alleviating the increasingly severe energy crisis. Seeking affordable, highly active, and stable photocatalysts is crucial to access the technology in a sustainable manner. Herein, a trivalent iron‐doped covalent triazine‐based framework (CTF‐1) was elaborately designed in this study to finely tune the band structure and photocatalytic activity of CTF‐1 for H 2 production. With optimal doping amount, Fe 10 /CTF‐1 exhibited a satisfying H 2 production activity of 1460 μmol h −1 g −1 , corresponding to 28‐fold enhancement compared with pure CTF‐1. The Fe 3+ doping is responsible for a remarkedly broadened visible‐light adsorption range, improved reduction ability and inhibited electron–hole recombination of CTF‐1. Specifically, the doped Fe 3+ could serve as photocatalytically active center and “electron relay” to accelerate charge separation and transformation. This study offers a feasible strategy to validly design and synthesize CTF‐based photocatalytic materials to efficiently utilize solar energy." @default.
- W3191729377 created "2021-08-16" @default.
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- W3191729377 date "2021-08-18" @default.
- W3191729377 modified "2023-10-16" @default.
- W3191729377 title "Band Gap Tuning of Covalent Triazine‐Based Frameworks through Iron Doping for Visible‐Light‐Driven Photocatalytic Hydrogen Evolution" @default.
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- W3191729377 doi "https://doi.org/10.1002/cssc.202101308" @default.
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