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- W3192022691 abstract "The heterostructure can remarkably boost the HER activity contributed by the re-distribution of interface charge and the resulting modification of interface hydrogen adsorption behavior. Rational heterostructure-design in electrocatalysts represents a promising approach toward high performance in the electrocatalytic hydrogen evolution reaction (HER). In specific, optimizing the H adsorption behavior at the surface/interface of heterostructure is of key importance to improve the catalytic performance. Herein, we demonstrate the construction of a heterostructure from a well-defined oxygen-bridged Co/Mo heterometallic zeolitic imidazolate framework (MOZ) as an efficient electrocatalyst for HER. The optimized hybrid exhibits high catalytic activity and stability in electrolytes with a wide pH range. Detailed XPS, XAS and theoretical studies reveal that the regulation of metal species can tailor the lattice of Mo 2 C within the hybrid and induce the formation of defect sites, which could not only induce surface charge transfer between the atoms and provide an additional active site, but also affect the H adsorption behavior at the interface of a heterostructure. This work provides an effective strategy to design a heterostructure with tailored active sites for energy conversion." @default.
- W3192022691 created "2021-08-16" @default.
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- W3192022691 date "2021-07-01" @default.
- W3192022691 modified "2023-10-16" @default.
- W3192022691 title "Engineering nanointerface of molybdenum-based heterostructures to boost the electrocatalytic hydrogen evolution reaction" @default.
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- W3192022691 doi "https://doi.org/10.1016/j.jechem.2020.10.004" @default.
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