Matches in SemOpenAlex for { <https://semopenalex.org/work/W3195320267> ?p ?o ?g. }
- W3195320267 endingPage "106459" @default.
- W3195320267 startingPage "106459" @default.
- W3195320267 abstract "An innovative lithium-sulfur (Li-S) battery technology is proposed that provides high energy density, fast charging, and mechanical flexibility. Via the rapid (30 min) one-pot reaction of elemental sulfur and vinyl phosphonic acid (VPA), SVPA microparticles containing dissimilar sulfur allotropes were developed. The spontaneous formation of wrinkles and pores on the particles facilitates electrolyte access and alleviates mechanical stress during battery cycling. The large surface area created by the ordered sulfur domains enhances lithium diffusion coefficients and facilitates polysulfide conversion kinetics in the Li-S cells, leading to a high discharge capacity of 1529 mAh·g−1 at 0.05 C and excellent rate performance (721 mAh·g−1 at 7 C). Additionally, owing to the inherent electrode porosity imparted by SVPA microparticles, a high areal capacity of ~5 mAh·cm−2 is obtained at increased cathode loadings. Abundant phosphonate moieties at the surfaces and interfaces of particles act as effective chemical anchors for lithium polysulfides, thereby mitigating the shuttle effects, which can prolong cycle lives at various C rates. The impressive properties of the SVPA microparticles are demonstrated for Li-S pouch cells, which exhibit stable operation under various deformations and highlight the SVPA microparticles as a promising candidate for next-generation Li-S batteries for wearable electronics" @default.
- W3195320267 created "2021-08-30" @default.
- W3195320267 creator A5042482017 @default.
- W3195320267 creator A5061544428 @default.
- W3195320267 date "2021-11-01" @default.
- W3195320267 modified "2023-10-14" @default.
- W3195320267 title "Thirty-minute synthesis of hierarchically ordered sulfur particles enables high-energy, flexible lithium-sulfur batteries" @default.
- W3195320267 cites W1811991547 @default.
- W3195320267 cites W1967174587 @default.
- W3195320267 cites W1983189738 @default.
- W3195320267 cites W1987722945 @default.
- W3195320267 cites W1995494909 @default.
- W3195320267 cites W2021102231 @default.
- W3195320267 cites W2028894825 @default.
- W3195320267 cites W2038956975 @default.
- W3195320267 cites W2043276052 @default.
- W3195320267 cites W2044820148 @default.
- W3195320267 cites W2049522172 @default.
- W3195320267 cites W2086639913 @default.
- W3195320267 cites W2104551659 @default.
- W3195320267 cites W2151207643 @default.
- W3195320267 cites W2226018809 @default.
- W3195320267 cites W2227799874 @default.
- W3195320267 cites W2261365795 @default.
- W3195320267 cites W2286910343 @default.
- W3195320267 cites W2291145446 @default.
- W3195320267 cites W2320402183 @default.
- W3195320267 cites W2371002555 @default.
- W3195320267 cites W2407625640 @default.
- W3195320267 cites W2510446028 @default.
- W3195320267 cites W2519452050 @default.
- W3195320267 cites W2557350354 @default.
- W3195320267 cites W2575735654 @default.
- W3195320267 cites W2580615030 @default.
- W3195320267 cites W2585398187 @default.
- W3195320267 cites W2614935634 @default.
- W3195320267 cites W2765725925 @default.
- W3195320267 cites W2766118708 @default.
- W3195320267 cites W2787696522 @default.
- W3195320267 cites W2807075808 @default.
- W3195320267 cites W2885383843 @default.
- W3195320267 cites W2885615162 @default.
- W3195320267 cites W2886920240 @default.
- W3195320267 cites W2896461491 @default.
- W3195320267 cites W2901776632 @default.
- W3195320267 cites W2905033312 @default.
- W3195320267 cites W2913959819 @default.
- W3195320267 cites W2947565373 @default.
- W3195320267 cites W2948650589 @default.
- W3195320267 cites W2972405169 @default.
- W3195320267 cites W2997405275 @default.
- W3195320267 cites W3004350510 @default.
- W3195320267 cites W3022575194 @default.
- W3195320267 cites W3023505431 @default.
- W3195320267 cites W3081739209 @default.
- W3195320267 cites W3108286492 @default.
- W3195320267 cites W3121830772 @default.
- W3195320267 doi "https://doi.org/10.1016/j.nanoen.2021.106459" @default.
- W3195320267 hasPublicationYear "2021" @default.
- W3195320267 type Work @default.
- W3195320267 sameAs 3195320267 @default.
- W3195320267 citedByCount "16" @default.
- W3195320267 countsByYear W31953202672021 @default.
- W3195320267 countsByYear W31953202672022 @default.
- W3195320267 countsByYear W31953202672023 @default.
- W3195320267 crossrefType "journal-article" @default.
- W3195320267 hasAuthorship W3195320267A5042482017 @default.
- W3195320267 hasAuthorship W3195320267A5061544428 @default.
- W3195320267 hasBestOaLocation W31953202671 @default.
- W3195320267 hasConcept C121332964 @default.
- W3195320267 hasConcept C127413603 @default.
- W3195320267 hasConcept C134018914 @default.
- W3195320267 hasConcept C147789679 @default.
- W3195320267 hasConcept C155672457 @default.
- W3195320267 hasConcept C159985019 @default.
- W3195320267 hasConcept C163258240 @default.
- W3195320267 hasConcept C171250308 @default.
- W3195320267 hasConcept C17525397 @default.
- W3195320267 hasConcept C185592680 @default.
- W3195320267 hasConcept C191897082 @default.
- W3195320267 hasConcept C192562407 @default.
- W3195320267 hasConcept C2777379467 @default.
- W3195320267 hasConcept C2777464112 @default.
- W3195320267 hasConcept C2778541603 @default.
- W3195320267 hasConcept C42360764 @default.
- W3195320267 hasConcept C49110097 @default.
- W3195320267 hasConcept C518881349 @default.
- W3195320267 hasConcept C555008776 @default.
- W3195320267 hasConcept C62520636 @default.
- W3195320267 hasConcept C6648577 @default.
- W3195320267 hasConcept C68801617 @default.
- W3195320267 hasConcept C71924100 @default.
- W3195320267 hasConcept C73916439 @default.
- W3195320267 hasConceptScore W3195320267C121332964 @default.
- W3195320267 hasConceptScore W3195320267C127413603 @default.
- W3195320267 hasConceptScore W3195320267C134018914 @default.
- W3195320267 hasConceptScore W3195320267C147789679 @default.
- W3195320267 hasConceptScore W3195320267C155672457 @default.