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- W3195639655 abstract "The stability of prototypical dislocation defects occurring in the ordered lamellar morphologies of block copolymers is of particular interest for both practical applications and fundamental research. Here, we study the impact of the segregation strength, compositional asymmetry, and architectural asymmetry on the evolution kinetics of single dislocation as well as the stability of its derivative disconnection defect occurring in the lamellar morphologies formed by AB diblock and AB2 miktoarm star copolymers using self-consistent field theory coupled with the string method and single-chain-in-mean-field simulations. Our results indicate that the segregation strength generally increases the stability of the two defects, whereas the two other factors of asymmetry lower the stability of the single dislocation and significantly enhance the stability of the single disconnection due to the effect of spontaneous curvature. In particular, the single disconnection becomes metastable and can survive for a long period at intermediate segregation and thus may be promisingly applicable for the fabrication of regularly broken lines." @default.
- W3195639655 created "2021-08-30" @default.
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- W3195639655 date "2021-08-17" @default.
- W3195639655 modified "2023-10-18" @default.
- W3195639655 title "Impact of Molecular Asymmetry of Block Copolymers on the Stability of Defects in Aligned Lamellae" @default.
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- W3195639655 doi "https://doi.org/10.1021/acs.macromol.1c01192" @default.
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