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• W3195887211 endingPage "2102978" @default.
• W3195887211 startingPage "2102978" @default.
• W3195887211 abstract "Solid composite electrolyte-based Li battery is viewed as one of the most competitive system for the next generation batteries; however, it is still restricted by sluggish ion diffusion. Fast ion transport is a characteristic of the polyethylene oxide (PEO) amorphous phase, and the mobility of Li+ is restrained by the coordination interaction within PEO and Li+. Herein, the design of applying functionalized carbon dots (CDs) with abundant surface features as fillers is proposed. High ionic conductivity is achieved in the CD-based composite electrolytes resulting from enhanced ion migration ability of polymer segments and mobility of Li+. Specially, the optimum effect with nitrogen and sulfur co-doped carbon dots (NS-CD) is a consequence of strong interaction between edge-nitrogen/sulfur in NS-CD and Li+. Solid-state nuclear magnetic resonance results confirm that more mobile Li+ is generated. Moreover, it is observed that lithium dendrite is suppressed compared to PEO electrolyte associated with reinforced mechanical properties and high transference number. The corresponding all-solid-state batteries, with the cathode of LiFePO4 or high voltage NCM523, exhibit long cycling life and excellent rate performances. It is a novel strategy to achieve high ionic conductivity composite electrolyte with uniform lithium deposition and provides a new direction to the mechanism of fast Li+ movement." @default.
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• W3195887211 date "2021-08-20" @default.
• W3195887211 modified "2023-10-16" @default.
• W3195887211 title "Carbon Dots Evoked Li Ion Dynamics for Solid State Battery" @default.
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• W3195887211 doi "https://doi.org/10.1002/smll.202102978" @default.
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