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• W3195996893 abstract "• Robust AFM correlations as a result of Co ions. • The role of Co ions in stabilizing the co-existing magnetic phases in double perovskite oxides. • A comparative magnetic phase diagram to illustrate the phase coexistence in Y 2 Ni x Co 1−x MnO 6 . We present a comparative study of double perovskites Y 2 Ni x Co 1−x MnO 6 for x = 1, 0.5, and 0. The polycrystalline samples of Y 2 Ni x Co 1−x MnO 6 with space group P2 1 /n were synthesized via sol-gel technique. X-ray photoelectron spectroscopy (XPS) confirms the presence of majority Ni 2+ /Mn 4+ in Y 2 NiMnO 6 (YNMO) and a mixed valence state Ni 2+/3+ /Co 2+/3+ /Mn 4+/3+ in co-doped Y 2 Ni 0.5 Co 0.5 MnO 6 (YNCMO). The temperature dependent magnetization results suggest homogeneous substitution of Ni ions with Co ions with minimal contribution of 3 + cationic magnetic interactions in YNCMO. The superexchange ferromagnetic (FM) interaction has a major contribution to the magnetism of YNMO. The strength of antiferromagnetic (AFM) coupling resulting from the antiphase boundaries in Y 2 Ni x Co 1−x MnO 6 increases with the increase in the Co concentration. The AC susceptibility (AC-χ) study further validates the presence of higher density of antiphase boundaries, which is reflected by the dynamics of domain walls in YNCMO. The isothermal magnetic entropy change (Δ S M ) as functions of temperature and magnetic field is exploited to assess the stabilization of different magnetic phases. The findings of Δ S M ( T ,µ 0 H ) lead to the proposed new magnetic phase diagrams for Y 2 Ni x Co 1−x MnO 6 for x = 1 and 0.5, in comparison with the previously established phase diagram of Y 2 CoMnO 6 ." @default.
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• W3195996893 date "2021-12-01" @default.
• W3195996893 modified "2023-10-12" @default.
• W3195996893 title "Competing magnetic interactions and emergent phase diagrams in double perovskite Y2NixCo1−xMnO6" @default.
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• W3195996893 doi "https://doi.org/10.1016/j.jallcom.2021.161624" @default.
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