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• W3196138268 abstract "The Ni self-diffusion in glass forming Pd40Ni40S20, Pd37Ni37S26 and Pd31Ni42S27 melts was probed by incoherent, quasielastic neutron scattering over a temperature range between 773 and 1023 K. The Ni self-diffusion coefficients are on a 10−10 m2 s−1–10−9 m2 s−1 scale and barely change with composition. Each composition exhibits an Arrhenius-type temperature dependence of the Ni self-diffusion coefficients, which results in activation energies ranging from EA = 348 ± 16 meV for Pd40Ni40S20 to EA = 387 ± 6 meV for Pd37Ni37S26. The structural relaxation shows a stretched exponential behavior even far above the liquidus temperatures. In addition, the viscosity of the Pd37Ni37S26 melt was measured under reduced gravity conditions. The diffusion calculated from the viscosity reveals a significant deviation from the measured Ni self-diffusion by a factor between 4 and 8. This may indicate a dynamic decoupling between the atoms within the Pd–Ni–S equilibrium melts." @default.
• W3196138268 created "2021-08-30" @default.
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• W3196138268 date "2021-08-18" @default.
• W3196138268 modified "2023-10-16" @default.
• W3196138268 title "Ni self-diffusion in glass forming Pd–Ni–S melts" @default.
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• W3196138268 doi "https://doi.org/10.1088/1361-648x/ac1968" @default.
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• W3196138268 hasPublicationYear "2021" @default.
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