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- W3196151208 abstract "Feasible strategies are desirable for preparing zeolitic nanosheets with opener porosities and more accessible active sites. Highly delaminated FER nanosheets (ECNU-17) with unit-cell scale thickness were hydrothermally synthesized using a simple, small, and low-cost imidazole molecule as the sole organic structure-directing agent (OSDA). The single OSDA directed the formation of the FER framework, while the π–π stacked OSDAs terminated the growth perpendicular to the zeolite sheets. The ECNU-17 nanosheet is only 2.9 nm in thickness, corresponding to one and a half FER unit cells along a-axis. With open hierarchical porosity and an enhanced external surface area of 253 m2 g–1, ECNU-17 is endowed with improved mass transport and a significantly increased number of active acid sites accessible to bulky organic molecules. The ultrathin sheets of ECNU-17 aluminosilicate display excellent activity and selectivity for the protection reaction of benzaldehyde with pentaerythritol as well as the cracking of 1,3,5-triisopropylbenzene." @default.
- W3196151208 created "2021-08-30" @default.
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- W3196151208 date "2021-08-25" @default.
- W3196151208 modified "2023-10-14" @default.
- W3196151208 title "Two Coexisting Forms of Simple Molecules for Directing Sesqui-Unit-Cell Zeolite Nanosheets" @default.
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- W3196151208 doi "https://doi.org/10.1021/acs.chemmater.1c01876" @default.
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