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• W3196182057 endingPage "28541" @default.
• W3196182057 startingPage "28535" @default.
• W3196182057 abstract "Direct conversion of CO2 to high value-added carbon products based on molten salt electrochemistry has been proven to be a feasible approach to solve the climate problem and achieve carbon neutrality. In this work, carbon nanotubes (CNTs), carbon spheres (CSs) and honeycomb carbon are synthesized by electrolysis of a single or multiple alkali metal carbonate electrolyte. The elemental composition, morphology and structure, crystallinity and graphitization degree of carbon products are characterized by electron dispersive spectroscopy (EDS), scanning electron microscopy (SEM), transmission electron microscope (TEM), X-ray diffraction (XRD) and Raman microspectroscopy (RAM). The results demonstrate that a high yield of CNTs is obtained in Li2CO3 electrolyte by regulating the electrolysis temperature and current density. Compared to pure Li2CO3, Li-Na carbonate electrolyte with 1 wt% stannic oxide/cerium oxide (SnO2/GeO2) favors CS formation rather than CNT formation. Additionally, honeycomb carbon products are generated in Li-Na-K electrolyte, when the electrolysis temperature is lower than 600 °C. Overall, this work provides a novel carbon neutral strategy where high value-added carbon products are synthesized using CO2 as a carbon source." @default.
• W3196182057 created "2021-08-30" @default.
• W3196182057 creator A5048861593 @default.
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• W3196182057 date "2021-01-01" @default.
• W3196182057 modified "2023-10-16" @default.
• W3196182057 title "Electrochemical conversion of CO₂ into value-added carbon with desirable structures <i>via</i> molten carbonates electrolysis" @default.
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• W3196182057 doi "https://doi.org/10.1039/d1ra03890g" @default.
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• W3196182057 hasPublicationYear "2021" @default.
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