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• W3196244617 endingPage "8431" @default.
• W3196244617 startingPage "8421" @default.
• W3196244617 abstract "Photoelectrochemical solar energy conversion offers a way to directly store light into energy-rich chemicals. Photoanodes based on the WO3/BiVO4 heterojunction are most effective mainly thanks to the efficient separation of photogenerated charges. The WO3/BiVO4 interfacial space region in the heterojunction is investigated here with the increasing thickness of the BiVO4 layer over a WO3 scaffold. On the basis of X-ray diffraction analysis results, density functional theory simulations show a BiVO4 growth over the WO3 layer along the BiVO4 {010} face, driven by the formation of a stable interface with new covalent bonds, with a favorable band alignment and band bending between the two oxides. This crystal facet phase matching allows a smooth transition between the electronic states of the two oxides and may be a key factor ensuring the high efficiency attained with this heterojunction. The photoelectrochemical activity of the WO3/BiVO4 photoanodes depends on both the irradiation wavelength and the thickness of the visible-light-absorbing BiVO4 layer, a 75 nm thick BiVO4 layer on WO3 being best performing." @default.
• W3196244617 created "2021-08-30" @default.
• W3196244617 creator A5005457843 @default.
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• W3196244617 date "2021-08-12" @default.
• W3196244617 modified "2023-10-12" @default.
• W3196244617 title "WO₃/BiVO₄ Photoanodes: Facets Matching at the Heterojunction and BiVO₄ Layer Thickness Effects" @default.
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• W3196244617 doi "https://doi.org/10.1021/acsaem.1c01623" @default.
• W3196244617 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8414527" @default.
• W3196244617 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34485843" @default.
• W3196244617 hasPublicationYear "2021" @default.
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