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• W3196993722 endingPage "12574" @default.
• W3196993722 startingPage "12560" @default.
• W3196993722 abstract "Herein, we report a sacrificial carbon fiber (CF) template-assisted synthesis of LiNi0.8Co0.15Al0.05O2 (C-NCA) by the Pechini method. An anisotropic primary particle morphology with an interconnected microstructure is obtained, originating from local overheating and oxygen-deficient zones induced by combustion of the CFs during high-temperature lithiation. Moreover, the particles assembled around the CFs demonstrated denser packing compared to the reference bare NCA (B-NCA) synthetized in the absence of the CF template. The anisotropic surfaces facilitate ion transport and stabilize the structure for high voltage and temperature operation. C-NCA||Li metal cells exhibit a reversible capacity of 106 mA h g–1 at 10 C and are able to retain 96% of their initial capacity as the C-rate is reverted to 0.1 C. The state of health of C-NCA||graphite full cells remains at 70% after 200 cycles at 0.33 C within 2.8–4.3 V. The results outperform the B-NCA cell, exhibiting a significant loss over 66 cycles while delivering only 50% of its initial capacity. The synthesis method allows for a straightforward route for tailoring the particle size, shape, and crystallinity, enabling the development of stable nickel-rich cathode materials, even at an upper cutoff voltage of 4.5 V or an operating temperature of 60 °C." @default.
• W3196993722 created "2021-09-13" @default.
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• W3196993722 date "2021-09-03" @default.
• W3196993722 modified "2023-10-09" @default.
• W3196993722 title "Improved Lithium-Ion Transport Within the LiNi_0.8Co_0.15Al_0.05O₂ Secondary Cathode Particles Through a Template-Assisted Synthesis Route" @default.
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• W3196993722 doi "https://doi.org/10.1021/acssuschemeng.1c03179" @default.
• W3196993722 hasPublicationYear "2021" @default.
• W3196993722 type Work @default.

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