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• W3197177629 abstract "In this paper, we report on the experimental determination of photon emission rates of laser-excited cobalt clusters, ${{mathrm{Co}}_{n}}^{+}$ ($n=5--23$), deduced from fragmentation mass spectrometry and metastable decay fractions. The rates are so high that they can only be ascribed to recurrent fluorescence (RF), a process where emitting states are populated by inverse internal conversion, followed by photon emission. Cooling via electronic states is confirmed by quantitative agreement with calculated rates using the low-lying electronic transitions predicted by time-dependent density functional theory calculations for $n=5--10$, which are performed considering all electrons and including relativistic effects implicitly. The outstanding agreement between experiment and theory provides clear evidence that the clusters radiate via electronic states, being a consistent theoretical and experimental study invoking RF." @default.
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• W3197177629 date "2021-09-08" @default.
• W3197177629 modified "2023-10-15" @default.
• W3197177629 title "Unravelling the electronic nature of the radiative cooling of cobalt clusters" @default.
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• W3197177629 doi "https://doi.org/10.1103/physrevresearch.3.033225" @default.
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