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• W3197201217 abstract "• Optimization of operational variables governing the SCWG of chicken manure. • Monitoring the quantitative results of optimized non-catalytic tests. • Preparation of activated carbon as a catalyst support using poultry farm residue. • Ceria effects on catalyst supports morphological characteristics. • Ni-supported catalyst preparation and its influence on hydrogen/syngas production. In recent years, supercritical water gasification has attracted the attention of scientists and environmentalists not only as an alternative method for direct disposal of poultry manure, but also as an efficient hydrogen-rich gas generation process. In this study, by varying the temperature (375–450 °C), residence time (5–35 min), and feed concentration (2.5–3.5 wt%), some non-catalytic supercritical water gasification tests were designed and carried out in a stainless-steel U-type batch reactor to assess the optimum operational condition. To stimulate hydrogen production, catalytic experiments were conducted using the optimized condition (450 °C, 15 min, and 2.5 wt% of feedstock). The prepared catalyst supports and final nanocatalysts (Ni/Activated carbon, Ni/activated carbon-CeO 2 nanorods) were then thoroughly characterized by various analytical instruments to verify the differences between the metal oxide-free and composite-like catalyst supports. Moreover, elemental analysis, gas and liquid chromatography were conducted to provide a deep understanding toward the impacts that composite-like catalyst support could have on diversity and quality of products. The experimental results revealed that, although in catalytic experiments the H 2 yields were higher than those recorded in non-catalytic experiments, highest hydrogen selectivity of 36.42 % could be achieved when Ni/activated carbon-CeO 2 nanorods were employed." @default.
• W3197201217 created "2021-09-13" @default.
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• W3197201217 date "2021-10-01" @default.
• W3197201217 modified "2023-09-29" @default.
• W3197201217 title "Hydrogen-rich gas production through supercritical water gasification of chicken manure over activated carbon/ceria-based nickel catalysts" @default.
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• W3197201217 doi "https://doi.org/10.1016/j.jaap.2021.105318" @default.
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