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- W3197232172 abstract "Porous three-dimensional (3D) assemblies of nanocarbons with large surface areas and tunable physical properties are attractive for a wide range of applications, such as energy storage electrodes, pollution adsorption, and thermal insulators. However, the full utilization of these materials is impeded by two challenges: forming 3D robust porous network structures that retain the intrinsic properties of the nanocarbon and achieving high shape-tunability to create structures with desired shapes. To address these challenges, gelatins with zwitterionic and hydrogen-bonded helical structure were considered a bio-derived binder to modulate the structural integrity of carbon nanotube (CNT) network which consists of overlapping nanotubes held by weak van der Waals attraction. The resulting CNT/gelatin wet-gels have favorable rheological properties, enabling 3D printing into complex porous architectures. Moreover, the 3D-printed complex wet-gel structure was successfully transformed into elastic and hierarchical porous structures consisting of micro-, meso-, and macro-scale pores with large specific surface areas of ∼988 m2 g−1 and excellent mechanical stability without permanent deformation even at 85% compressive strain. The resulting high shape-tunability, high elasticity, and large surface area are attributed to the reinforcement of the existing nanotube cross-linking points strengthened by the gelatin-derived graphitic layer coating without deteriorating the intrinsic properties of CNTs." @default.
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- W3197232172 date "2021-10-01" @default.
- W3197232172 modified "2023-09-26" @default.
- W3197232172 title "The shape tunable gelatin/carbon nanotube wet-gels for complex three-dimensional cellular structures with high elasticity" @default.
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- W3197232172 doi "https://doi.org/10.1016/j.carbon.2021.08.086" @default.
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