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- W3197341159 abstract "Biomass-templated biomimetic mineralization has recently emerged as a readily scalable method for the fabrication of mesoporous metal oxides due to the wide availability of the templates and their delicate hierarchical porous nanostructures. However, the selective ionic interactions of biomass-derived templates limit the possible chemical compositions of the desired products. Polyphenols can potentially introduce more general ionic adsorption to biomass-derived templates through the self-assembly of metal-phenolic networks (MPNs), leading to successful synthesis of a much broader range of mesoporous materials. As an illustration of this strategy, we designed a novel method for the fabrication of hierarchical mesoporous bimetallic hybrid nanocatalysts through calcination of biomass collagen-templated bimetallic MPNs. The resultant Bi/Ti bimetallic hybrid nanocatalysts inherited the hierarchical mesostructures of their collagen templates and showed excellent photocatalytic performance in the visible-light region (420−700 nm), which was consistent with the theoretical calculations using the first-principles density function theory. This simple and low-cost MPN-based approach possibly provides a universal platform for stable mineralization of biomass templates, paving the avenue towards a wide range of potential applications in environmental-friendly synthesis of mesoporous metal oxide materials." @default.
- W3197341159 created "2021-09-13" @default.
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- W3197341159 date "2021-11-01" @default.
- W3197341159 modified "2023-10-17" @default.
- W3197341159 title "Bi/Ti-phenolic network induced biomimetic synthesis of mesoporous hierarchical bimetallic hybrid nanocatalysts with enhanced visible-light photocatalytic performance" @default.
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- W3197341159 doi "https://doi.org/10.1016/j.colsurfa.2021.127518" @default.
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