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• W3197465173 endingPage "111994" @default.
• W3197465173 startingPage "111994" @default.
• W3197465173 abstract "A heterogeneous electro-Fenton (hetero-EF) system can effectively broaden the applicable pH range, although the decreased electrogeneration efficiency of H2O2 at elevated pH (especially neutral conditions) is unfavorable for the efficient removal of organic pollutants. Herein, a tannic acid-Fe complex derivative-modified carbon felt (TFD@CF) cathode was prepared for hetero-EF treatment of organic pollutants over a wide pH range. Interestingly, the as-prepared hetero-EF cathode could act as a pH regulator that acidified the solution over a wide pH range. As expected, the TFD@CF cathode exhibited excellent hetero-EF activity for the removal of diverse organic pollutants (such as methyl orange, methylene blue, sulfamerazine, bisphenol A and 2,4-dichlorophenoxyacetic acid) at neutral and even alkaline pH (removal efficiency >90 %). A total of 2.98 kWh kg-1 COD-1 with 83.2 % COD removal could be achieved by the TFD@CF cathode for the treatment of actual textile dyeing secondary wastewater. Electrochemical characterizations proved that the TFD@CF cathode had excellent electrochemical properties with improved electron transfer ability and a well-pronounced Fe(III) electroreductive response. Meanwhile, more acidic groups were newly generated during the electrochemical reaction (an increase of 30.1 %), thus dissociating more H+ into solution. The identification of reactive oxygen species suggested that OH and 1O2 could be responsible for the removal of organic pollutants in the TFD@CF EF system. These interesting findings may provide new insights into the design of multifunctional hetero-EF cathodes for the removal of refractory organic pollutants." @default.
• W3197465173 created "2021-09-13" @default.
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• W3197465173 date "2022-03-01" @default.
• W3197465173 modified "2023-09-27" @default.
• W3197465173 title "Tannic acid-Fe complex derivative-modified electrode with pH regulating function for environmental remediation by electro-Fenton process" @default.
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• W3197465173 doi "https://doi.org/10.1016/j.envres.2021.111994" @default.
• W3197465173 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34487696" @default.
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