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• W3197580397 abstract "The performance of a sodium-ion (Na) battery is significantly influenced by its electrolyte characteristics. In particular, the transport properties of the electrolyte have considerable effects on the discharge rate capability. During discharging of a Na battery at high current densities, a concentration gradient of Na salt develops because both cations and anions are mobile in the liquid electrolyte. Concentration polarization can be suppressed by increasing the Na+ transference number (tNa+) of the electrolyte. This study demonstrates that highly concentrated NaN(SO2F)2 dissolved in 3-methylsulfolane (MSL) exhibits a high tNa+ value of >0.6 under anion-blocking conditions. Raman spectroscopy revealed that Na+ ions formed complexes with MSL and anions in the electrolyte. Na+ ions exchange ligands dynamically and move faster than the ligands, resulting in a high tNa+. The high tNa+ enables a high-rate discharge of the Na battery, despite the low ionic conductivity of the highly concentrated electrolyte." @default.
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• W3197580397 date "2021-11-05" @default.
• W3197580397 modified "2023-10-12" @default.
• W3197580397 title "Highly Concentrated NaN(SO₂F)₂/3-Methylsulfolane Electrolyte Solution Showing High Na-Ion Transference Number under Anion-Blocking Conditions" @default.
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• W3197580397 doi "https://doi.org/10.5796/electrochemistry.21-00095" @default.
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