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- W3197831154 endingPage "122540" @default.
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- W3197831154 abstract "Two new Pb(II) coordination polymers, namely, [Pb(Hpydc)2]n (1), [Pb(Hpydc)2(H2O)]n·2n(H2O) (2) (H2pydc = 2,5-pyridinedicarboxylic acid) have been prepared by the reaction of PbCl2 with pyridinedicarboxylic acid and fully characterized. Compound 1 contains ‘sql’ topological layers built from one-dimensional (1D) Pb-carboxylate infinite chains, and the layers are further packed into a 3D architecture by strong hydrogen bonds interactions. Compound 2 consists of 1D infinite chains containing Pb-dimers. The 3D supramolecular Pb(II) coordination complex of 2 is created by π – π interactions between the pyridine rings of the Hpydc ligands. In addition, solid-state properties of thermal stability and fluorescence for these crystalline materials are also presented. Time-dependent density functional theory (TDDFT) calculations reveal that the mechanism of the fluorescence emissions are dominantly resulted from the ligand-to-metal charge transfer (LMCT) and partial the intraligand π→π∗ and/or n→π∗ transitions for 1 and 2, which are in good agreement with their fluorescence spectra and crystal structure." @default.
- W3197831154 created "2021-09-13" @default.
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- W3197831154 date "2021-11-01" @default.
- W3197831154 modified "2023-10-16" @default.
- W3197831154 title "Synthesis, structures and properties of lead coordination polymers based on pyridinedicarboxylate ligand" @default.
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- W3197831154 doi "https://doi.org/10.1016/j.jssc.2021.122540" @default.
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