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- W3198295912 abstract "A green and environmentally friendly route uses air to fabricate the hollow structured nanocomposites, which successfully self-assembled the uniform MoO 3 nanodots (denote as MoO 3 NDs, about 1.8 nm) into the mesoporous SiO 2 hollow nanosphere (denote as MoO 3 /SiO 2 HN) in a homogeneous solution. The new type of NDs-supported nanocomposite is fully characterized with different techniques (XPS, NH 3 -TPD, EPR, EIS and UV–vis). The result is that the small size of NDs enhances the number of active sites exposed on the surface of the carrier or mesoporous channels, and the novel catalyst of MoO 3 /SiO 2 HN exhibits rapid electron transfer capabilities and abundant O-vacancies. Besides, the possible mechanism of desulfurization reaction has also been studied in detail. It is found that the O-vacancy of the catalyst facilitates the adsorption of H 2 O 2 and the rapid electron transfer of NDs promotes decomposition of H 2 O 2 to produce more active oxygen (O - ), thereby improving the catalytic oxidation desulfurization performance. • Mesoporous MoO 3 /SiO 2 HN were successfully self-assembled in homogeneous solution. • MoO 3 /SiO 2 HN material displayed rapid electron transfers and abundant O-vacancies. • Novel MoO 3 /SiO 2 HN catalyst owned excellent catalytic desulfurization performance. • The surface rapid electron transfers and abundant O-vacancies played important roles in the desulfurization reaction." @default.
- W3198295912 created "2021-09-13" @default.
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- W3198295912 date "2021-10-01" @default.
- W3198295912 modified "2023-09-29" @default.
- W3198295912 title "Facile synthesis of MoO3 nanodots self-assembled into hollow mesoporous silica: Enhancing efficient oxidative desulfurization and investigating reaction mechanism" @default.
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- W3198295912 doi "https://doi.org/10.1016/j.jece.2021.106309" @default.
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