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• W3198932750 endingPage "25074" @default.
• W3198932750 startingPage "25068" @default.
• W3198932750 abstract "Porous materials for C2 H2 /CO2 separation mostly suffer from high regeneration energy, poor stability, or high cost that largely dampen their industrial implementation. A desired adsorbent should have an optimal balance between excellent separation performance, high stability, and low cost. We herein report a stable, low-cost, and easily scaled-up aluminum MOF (CAU-10-H) for highly efficient C2 H2 /CO2 separation. The suitable pore confinement in CAU-10-H can not only provide multipoint binding interactions with C2 H2 but also enable the dense packing of C2 H2 inside the pores. This material exhibits one of the highest C2 H2 storage densities of 392 g L-1 and highly selective adsorption of C2 H2 over CO2 at ambient conditions, achieved by a low C2 H2 adsorption enthalpy (27 kJ mol-1 ). Breakthrough experiments confirm its exceptional separation performance for C2 H2 /CO2 mixtures, affording both large C2 H2 uptake of 3.3 mmol g-1 and high separation factor of 3.4. CAU-10-H achieves the benchmark balance between separation performance, stability, and cost for C2 H2 /CO2 separation." @default.
• W3198932750 created "2021-09-27" @default.
• W3198932750 creator A5007649916 @default.
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• W3198932750 creator A5039508546 @default.
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• W3198932750 creator A5050734459 @default.
• W3198932750 creator A5073926976 @default.
• W3198932750 creator A5083206827 @default.
• W3198932750 date "2021-10-20" @default.
• W3198932750 modified "2023-10-11" @default.
• W3198932750 title "Dense Packing of Acetylene in a Stable and Low‐Cost Metal–Organic Framework for Efficient C ₂ H ₂ /CO ₂ Separation" @default.
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