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• W3199529726 endingPage "2397" @default.
• W3199529726 startingPage "2380" @default.
• W3199529726 abstract "Understanding of the fundamental chemical and physical processes that lead to the formation and evolution of secondary organic aerosol (SOA) in the atmosphere has been rapidly advancing over the past decades. Many of these advancements have been achieved through laboratory studies, particularly SOA studies conducted in environmental chambers. Results from such studies are used to develop simplified representations of SOA formation in regional- and global-scale air quality models. Although it is known that there are limitations in the extent to which laboratory experiments can represent the ambient atmosphere, there have been no systematic surveys of what defines atmospheric relevance in the context of SOA formation. In this work, GEOS-Chem version 12.3 was used to quantitatively describe atmospherically relevant ranges of chemical and meteorological parameters critical for predictions of the mass, composition, and physical properties of SOA. For some parameters, atmospherically relevant ranges are generally well represented in laboratory studies. However for other parameters, significant gaps exist between atmospherically relevant ranges and typical laboratory conditions. For example, cold winter (less than 0 °C) and humid (greater than 70% RH) conditions are relatively common on the Earth’s surface but are poorly represented in published chamber data. Furthermore, the overlap in relative humidity and organic aerosol mass between chamber studies and ambient conditions is almost nonexistent. For parameters with significant gaps, extended laboratory studies and/or mechanistic models are needed to bridge these gaps." @default.
• W3199529726 created "2021-09-27" @default.
• W3199529726 creator A5019818769 @default.
• W3199529726 creator A5042689433 @default.
• W3199529726 creator A5081595136 @default.
• W3199529726 date "2021-07-14" @default.
• W3199529726 modified "2023-10-17" @default.
• W3199529726 title "Quantifying Atmospheric Parameter Ranges for Ambient Secondary Organic Aerosol Formation" @default.
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• W3199529726 doi "https://doi.org/10.1021/acsearthspacechem.1c00090" @default.
• W3199529726 hasPublicationYear "2021" @default.
• W3199529726 type Work @default.
• W3199529726 sameAs 3199529726 @default.

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