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- W3200214779 abstract "The design of artificially engineered chiral structures has received much attention, but the implementation of dynamic functions to modulate the chiroptical response of the systems is less explored. Here, we present a light-responsive G-quadruplex (G4)-based assembly in which chirality enrichment is induced, tuned, and fueled by molecular switches. In particular, the mirror-image dependence on photoactivated azo molecules, undergoing trans-to-cis isomerization, shows chiral recognition effects on the inherent flexibility and conformational diversity of DNA G4s having distinct handedness (right- and left-handed). Through a detailed experimental and computational analysis, we bring compelling evidence on the binding mode of the photochromes on G4s, and we rationalize the origin of the chirality effect that is associated with the complexation event." @default.
- W3200214779 created "2021-09-27" @default.
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- W3200214779 date "2021-09-23" @default.
- W3200214779 modified "2023-09-30" @default.
- W3200214779 title "Light-Induced Modulation of Chiral Functions in G-Quadruplex–Photochrome Systems" @default.
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- W3200214779 doi "https://doi.org/10.1021/acs.jpclett.1c02207" @default.
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