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• W3200219982 endingPage "2107181" @default.
• W3200219982 startingPage "2107181" @default.
• W3200219982 abstract "Modulating the morphology and chemical composition is an efficient strategy to enhance the catalytic activity for water splitting, since it is still a great challenge to develop a bifunctional catalyst for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) over a wide pH range. Herein, Pd/NiFeOx nanosheets are synthesized with tightly arranged petal nanosheets and uniform mesoporous structure on nickel foam (NF). The porous 2D structure yields a larger surface area and exposes more active sites, facilitating water splitting at all pH values. The overpotential of Pd/NiFeOx nanosheets for OER is only 180, 169, and 310 mV in 1 m KOH, 0.5 m H2SO4, and 1 m phosphate-buffered saline (PBS) conditions at 10 mA cm−2 current density, as well as excellent HER activity with ultralow overpotential in a wide pH range. When using porous Pd/NiFeOx nanosheets as bifunctional catalysts for water splitting, it just required a cell voltage of 1.57 V to reach a current density of 20 mA cm−2 with nearly 100% faradic efficiency in alkaline conditions, which is much lower than that of benchmark Pt/CǁRuO2 (1.76 V) couples, along with the improving stability benefiting from the good corrosion resistance of the inner NiFeOx nanosheets." @default.
• W3200219982 created "2021-09-27" @default.
• W3200219982 creator A5015039046 @default.
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• W3200219982 creator A5067507847 @default.
• W3200219982 creator A5074516665 @default.
• W3200219982 creator A5076770005 @default.
• W3200219982 creator A5085352453 @default.
• W3200219982 date "2021-09-17" @default.
• W3200219982 modified "2023-10-14" @default.
• W3200219982 title "Porous Pd/NiFeO _x Nanosheets Enhance the pH‐Universal Overall Water Splitting" @default.
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• W3200219982 doi "https://doi.org/10.1002/adfm.202107181" @default.
• W3200219982 hasPublicationYear "2021" @default.
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