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• W3200327129 abstract "The stability, versatility, and reusability of an adsorbent are of great significance to its practicability to remove antibiotics from water due to their universal residual. Herein, a magnetic composite of nano-iron wrapped by graphitic carbon in the carbonaceous matrix with hierarchical pores (Fein/C-700) was constructed by one-step pyrolysis using Fein/Zn-MOF as a precursor. Fein/C-700 exhibited a core–shell structure and superparamagnetism behavior, which showed excellent chlortetracycline (CTC) adsorption with the maximum adsorption capacity of 546.5 mg/g. The adsorption process matched well with the pseudo-second-order kinetics model and Langmuir model, indicating chemisorption was likely contributed to the CTC adsorption. Electrostatic interaction, surface complexation, hydrogen bond, and π-π EDA interaction were the dominant driving forces. Cl- and SO42- significantly enhanced the CTC adsorption due to the electrostatic attraction or hydrogen bond formed among Fein/C-700, anions, and CTC. Fein/C-700 maintained high adsorption capacities in the mixed antibiotic system (255.1, 143.3, and 169.6 mg/g for CTC, ciprofloxacin, and sulfamethoxazole), in actual water (372.9, 383.3, 390.6, and 366.7 mg/g for CTC in Pearl River water, lake water, tap water, and ultrapure water), and regeneration (366.7, 354.2, 360.4, 314.6, and 301.0 mg/g for CTC in five runs), indicating a promising reusable adsorbent for the remediation of antibiotics in water. These findings provide a feasible and straightforward strategy to synthesize high stable magnetic nanoparticles derived from MOFs." @default.
• W3200327129 created "2021-09-27" @default.
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• W3200327129 date "2021-12-01" @default.
• W3200327129 modified "2023-09-27" @default.
• W3200327129 title "Nano-iron wrapped by graphitic carbon in the carbonaceous matrix for efficient removal of chlortetracycline" @default.
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• W3200327129 doi "https://doi.org/10.1016/j.seppur.2021.119693" @default.
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