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• W3200697361 abstract "The functionalization of an imine-based layered covalent organic framework (COF), containing phenanthroline units as ligands, has allowed the obtention of a heterobimetallated material. Photoactive Ir and Ni fragments were immobilized within the porous structure of the COF, enabling heterogeneous light-mediated Csp3–Csp2 cross-couplings. As radical precursors, potassium benzyl- and alkoxy-trifluoroborates, organic silicates, and proline derivatives were employed, which brings out the good versatility of Ir,Ni@Phen-COF. Moreover, in all the studied cases, an enhanced activity and stability have been observed in comparison with analogous homogenous systems." @default.
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• W3200697361 date "2021-09-21" @default.
• W3200697361 modified "2023-10-17" @default.
• W3200697361 title "Photoredox Heterobimetallic Dual Catalysis Using Engineered Covalent Organic Frameworks" @default.
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• W3200697361 doi "https://doi.org/10.1021/acscatal.1c03634" @default.
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