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- W3200803385 abstract "A new type of pyrene-based ammonium bromides (PABs) was synthesized via the reaction of bromomethyl pyrene and tertiary amines with different alkyl chains combined with graphitic carbon nitride (g-C3N4) through π-π stacking interactions. The new pyrene-based ammonium bromides were investigated both in homogenous phase and heterogeneous phase combining with g-C3N4 for the CO2 fixation reaction of epoxides under mild conditions. Obviously, the combination was proved to be an efficient system for the conversion of epoxides. The interaction between g-C3N4 and PABs was confirmed by quantum chemical calculations. g-C3N4/Py-C12 exhibited an excellent yield of cyclic carbonates (above 93%) at 80 °C, atmospheric pressure and solvent-free conditions. A preliminary kinetic study was performed using g-C3N4/Py-C12 and the activation energy was calculated to be 61.5 kJ mol-1." @default.
- W3200803385 created "2021-09-27" @default.
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- W3200803385 date "2021-01-01" @default.
- W3200803385 modified "2023-10-17" @default.
- W3200803385 title "Pyrene-based ammonium bromides combined with g-C<sub>3</sub>N<sub>4</sub> for the synergistically enhanced fixation reaction of CO<sub>2</sub> and epoxides" @default.
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- W3200803385 doi "https://doi.org/10.1039/d1ra05328k" @default.
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