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- W3200909246 abstract "Delineating intricate interactions between highly reactive Li-metal electrodes and the diverse constituents of battery electrolytes has been a long-standing scientific challenge in materials design for advanced energy storage devices. Here, we isolated lithium polysulfide anions (LiS4–) from an electrolyte solution based on their mass-to-charge ratio and deposited them on Li-metal electrodes under clean vacuum conditions using ion soft landing (ISL), a highly controlled interface preparation technique. The molecular level precision in the construction of these model interfaces with ISL, coupled with in situ X-ray photoelectron spectroscopy and ab initio theoretical calculations, allowed us to obtain unprecedented insight into the parasitic reactions of well-defined polysulfides on Li-metal electrodes. Our study revealed that the oxide-rich surface layer, which is amenable to direct electron exchange, drives multielectron sulfur oxidation (S0 → S6+) processes. Our results have substantial implications for the rational design of future Li–S batteries with improved efficiency and durability." @default.
- W3200909246 created "2021-09-27" @default.
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- W3200909246 date "2021-09-22" @default.
- W3200909246 modified "2023-10-17" @default.
- W3200909246 title "Role of Polysulfide Anions in Solid-Electrolyte Interphase Formation at the Lithium Metal Surface in Li–S Batteries" @default.
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- W3200909246 doi "https://doi.org/10.1021/acs.jpclett.1c01930" @default.
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