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• W3201055239 abstract "Demands for IR birefringent materials are increasing due to the rapid developments of IR laser applications. Herein, two new chain tellurides β-BaGa2Te4 and Ba5Ga2Ge3Te12 have been discovered. β-BaGa2Te4 crystallizes in the orthorhombic space group Imma (no. 74) with unit cell constants of a = 23.813(3) Å, b = 11.9673(19) Å, and c = 6.7215(9) Å, while Ba5Ga2Ge3Te12 crystallizes in the monoclinic space group P21/c (no. 14) with unit cell constants of a = 13.6540(3) Å, b = 9.6705(2) Å, and c = 23.1134(7) Å. The structure of β-BaGa2Te4 can be considered to be the antiparallel arrangement of one-dimensional (1D) [GaTe2] chains formed by edge-sharing GaTe4 tetrahedra, which are separated by Ba2+ cations. In the crystal structure of Ba5Ga2Ge3Te12, two kinds of 1D chains, namely chain 1 ∞1[(GaGe)3Te8] and chain 2 ∞1[(GaGe)2Te4], are stacked alternately and put together by the coulomb force with Ba2+ cations. In addition, First-principles calculations indicate that β-BaGa2Te4 has a large birefringence, ∼0.325 at 2050 nm, derived from the superposition of the polarizabilities of GaTe4 tetrahedra, implying that it has potential as an IR birefringent material. This work may provide some guidance for exploring new IR birefringent crystals." @default.
• W3201055239 created "2021-09-27" @default.
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• W3201055239 date "2021-09-16" @default.
• W3201055239 modified "2023-10-01" @default.
• W3201055239 title "Synthesis and Characterizations of Two Tellurides β-BaGa₂Te₄ and Ba₅Ga₂Ge₃Te₁₂ with Flexible Chain Structure" @default.
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• W3201055239 doi "https://doi.org/10.1021/acs.inorgchem.1c02045" @default.
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• W3201055239 hasPublicationYear "2021" @default.
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