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• W3201130257 abstract "Chemical looping reforming of methane coupled with CO2 reduction is a novel and useful route for methane conversion and CO2 reduction. The choice of oxygen carrier with high reactivity and strong resistance to carbon deposition is the key issue for this process. In this study, a series of LaxCe1–xFexNi1–xO3 oxides are used as oxygen carriers. The doping amounts of Ce and Ni ions have an influence on the reactivity of LaxCe1–xFexNi1–xO3. The calcination temperature also plays an important role in the performance of oxygen carrier during the chemical looping process. With an increase of calcination temperature, larger amounts of Ni species would immigrate to the surface of LaxCe1–xFexNi1–xO3 oxygen carrier. The amount of Ni species has an effect on the formation of carbon deposition. During the successive redox cycles, both La0.6Ce0.4Fe0.6Ni0.4O3-750 and La0.6Ce0.4Fe0.6Ni0.4O3-800 exhibit appropriate H2/CO ratios near 2.0. The H2/CO molar ratios of La0.6Ce0.4Fe0.6Ni0.4O3-850 and La0.6Ce0.4Fe0.6Ni0.4O3-900 increase sharply to much higher values (>2.0) with the cycle number, indicating the formation of carbon deposition. The result demonstrates that the La0.6Ce0.4Fe0.6Ni0.4O3 oxygen carrier calcined at lower temperature could enhance the resistance to carbon deposition." @default.
• W3201130257 created "2021-09-27" @default.
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• W3201130257 date "2021-09-10" @default.
• W3201130257 modified "2023-10-17" @default.
• W3201130257 title "Enhanced Resistance to Carbon Deposition over La<i>_x</i>Ce_1–<i>x</i>Fe<i>_x</i>Ni_1–<i>x</i>O₃ Oxygen Carrier for Chemical Looping Reforming" @default.
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• W3201130257 doi "https://doi.org/10.1021/acs.energyfuels.1c01932" @default.
• W3201130257 hasPublicationYear "2021" @default.
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