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• W3201161700 endingPage "9428" @default.
• W3201161700 startingPage "9422" @default.
• W3201161700 abstract "In the areas of condensed matter physics, geoscience, material science, and inorganic chemistry, how the crystal structures evolve under an external field such as high-pressure is a fundamental question. By taking TiSe2 as the case, we investigate the phase transformations of the layered transition-metal dichalcogenides (TMDs) under high-pressure. The ambient 6-fold P-3m1 TiSe2 undergoes a transformation into the monoclinic 8-fold coordinated C2/m phase at 15 GPa and then into the hexagonal 9-fold Fe2P-type structure at 34 GPa. The above phase transitions can be unitedly described as the evolution of the vacancies: from a layered structure with two-dimensional (2D) vacancies to the structure with one-dimensional (1D) and zero-dimensional (0D) vacancies. The proposed densification model of TiSe2 reveals the processes how the symmetry breaking phase of spatial chemical bonding restores the symmetry under the isotropic external pressure." @default.
• W3201161700 created "2021-09-27" @default.
• W3201161700 creator A5002873170 @default.
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• W3201161700 date "2021-09-23" @default.
• W3201161700 modified "2023-10-16" @default.
• W3201161700 title "From Two-, One-, to Zero-Dimensional Vacancies: A Densification Pattern for a Typcial Transition-Metal Dichalcogenide of TiSe₂" @default.
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• W3201161700 doi "https://doi.org/10.1021/acs.jpclett.1c02308" @default.
• W3201161700 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34553935" @default.
• W3201161700 hasPublicationYear "2021" @default.
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