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- W3201202223 endingPage "106538" @default.
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- W3201202223 abstract "Constructing ternary structure is one of the most effective design strategies to break the efficiency ceiling of traditional binary organic solar cells (OSCs). Here, a new Y-series non-fullerene acceptor (Y-T) featuring 1,3-diethyl-2-thiobarbituric acid (DTBA) end groups is developed as a third component for the classical PM6:Y6 binary system. The champion power conversion efficiency of ternary OSCs is increased from 15.64% to 17.37% via incorporating 10 wt% Y-T, with the simultaneously enhanced open-circuit voltage (Voc) of 0.865 V, a short-circuit current density (Jsc) of 26.90 mA/cm2, and a fill factor (FF) of 74.97%. The positive contribution of Y-T in the ternary blend can be ascribed to the improved spectroscopic complementarity and enhanced exciton utilization ratio due to the additional energy transfer process. Moreover, Y-T guest acceptor plays a critical role in adjusting the active layer morphology and facilitating three-dimension phase separation, resulting in a balanced charge transport and enhanced FF of ternary OSCs. This work provides insight into the molecular design of non-fullerene acceptor and suggest guidelines to rationally select guest component for ternary OSCs." @default.
- W3201202223 created "2021-09-27" @default.
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- W3201202223 date "2021-12-01" @default.
- W3201202223 modified "2023-10-18" @default.
- W3201202223 title "Boosting photovoltaic performance of ternary organic solar cells by integrating a multi-functional guest acceptor" @default.
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- W3201202223 doi "https://doi.org/10.1016/j.nanoen.2021.106538" @default.
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