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- W3201231789 abstract "Electrosynthesis of hydrogen peroxide (H2O2) in the acidic environment could largely prevent its decomposition to water, but efficient catalysts that constitute entirely earth-abundant elements are lacking. Here we report the experimental demonstration of narrowing the interlayer gap of metallic cobalt diselenide (CoSe2), which creates high-performance catalyst to selectively drive two-electron oxygen reduction toward H2O2 in an acidic electrolyte. The enhancement of the interlayer coupling between CoSe2 atomic layers offers a favorable surface electronic structure that weakens the critical *OOH adsorption, promoting the energetics for H2O2 production. Consequently, on the strongly coupled CoSe2 catalyst, we achieved Faradaic efficiency of 96.7 %, current density of 50.04 milliamperes per square centimeter, and product rate of 30.60 mg cm−2 h−1. Moreover, this catalyst shows no sign of degradation when operating at −63 milliamperes per square centimeter over 100 hours." @default.
- W3201231789 created "2021-09-27" @default.
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- W3201231789 date "2021-10-20" @default.
- W3201231789 modified "2023-10-16" @default.
- W3201231789 title "Strongly Coupled Cobalt Diselenide Monolayers for Selective Electrocatalytic Oxygen Reduction to H <sub>2</sub> O <sub>2</sub> under Acidic Conditions" @default.
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- W3201231789 doi "https://doi.org/10.1002/ange.202111075" @default.
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