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• W3201380919 abstract "Owing to the insoluble organosulfur mechanism and stable cycling life, sulfurized polyacrylonitrile (SPAN) developed as a promising cathode material for high-energy potassium–sulfur batteries (KSBs). However, it is yet a major challenge to achieve fast catalytic kinetics and high reversible capacity in SPAN-based cathodes. Here, one-step electrospun SPAN nanofibers embedded with Fe[Formula: see text]Nb[Formula: see text]O metal oxide nanoparticles (FeNb@SPAN) have been successfully developed to construct sulfur electrodes with high electrochemical activity, high sulfur utilization, and high cycling stability. The as-prepared freestanding FeNb@SPAN composite cathode, which featuring interwoven nanofibers with Fe[Formula: see text]Nb[Formula: see text]O nanoparticles homogeneously implanted, possesses high storage space for volume expansion and suppresses polysulfide dissolution during potassiation/depotassiation. Benefiting from its unique structure and composition in electrode design, the FeNb@SPAN cathode is endowed with outstanding energy storage performances with a high initial specific capacity of 776 mAh [Formula: see text] g[Formula: see text] under 50 mA [Formula: see text] g[Formula: see text] and an excellent cycling capability of 201 mAh [Formula: see text] g[Formula: see text] after 80 charge/discharge processes. This work heralds a feasible strategy toward SPAN-based sulfur host materials in the structural design of next-generation high-performance cathode materials for KSBs and other metal–sulfur batteries." @default.
• W3201380919 created "2021-09-27" @default.
• W3201380919 creator A5000838895 @default.
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• W3201380919 date "2021-09-23" @default.
• W3201380919 modified "2023-09-26" @default.
• W3201380919 title "An <i>in-situ</i> catalytic-insoluble strategy enabled by sulfurized polyacrylonitrile-based composite cathode for potassium–sulfur batteries" @default.
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• W3201380919 doi "https://doi.org/10.1142/s1793604721430037" @default.
• W3201380919 hasPublicationYear "2021" @default.
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