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• W3201416458 abstract "• Synthesis of zeolites with different Na2O/SiO2 ratios as an index of zeolite hydrophobicity. • Using synthesized zeolites in synergy with a plasma system for tetracycline degradation. • Study on the effect of plasma and operational parameters. • Study on conversion of H 2 O 2 and O 3 to active radicals in hybrid zeolite-plasma system. • Study on role of • OH and O 2 •− in degradation of tetracycline in plasma-zeolite system. • Proposing a mechanism for tetracycline degradation in the hybrid system. In this work, a combination of synthesized zeolite with a Dielectric Barrier Discharge (DBD) air plasma reactor was applied for the removal of tetracycline (TC) from effluents. The zeolites with different Na 2 O/SiO 2 ratios were synthesized and inserted in a DBD reactor. The as-prepared zeolites were characterized by FTIR, SEM, BET, EDX, XRD, and TEM. The XRD results showed that the P-type zeolite turned to Y-type zeolite with an increasing Na 2 /SiO 2 ratio from 0.5 to 1.5 and 2.5. The TC degradation experiments indicated that 79.1% of the initial TC was removed from the solution by the hybrid plasma- zeolite (Na 2 O/SiO 2 ratio of 0.5) system after 45 min. The plasma in synergy with zeolite caused the changing amount of long-life oxidants in the system and converted it to higher reactive species. The combined system could reduce around 17 and 10% of the total organic carbon (TOC) and chemical oxygen demand (COD) more than the sole DBD system, respectively. Losing just 8% of the initial efficiency of the hybrid system after four successive runs revealed the stability of the proposed system. The radical trapping experiment method indicated that the role of • OH in the TC degradation was more critical than that of O 2 •− ." @default.
• W3201416458 created "2021-09-27" @default.
• W3201416458 creator A5064505369 @default.
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• W3201416458 date "2021-12-01" @default.
• W3201416458 modified "2023-10-17" @default.
• W3201416458 title "Tetracycline degradation using combined system of dielectric barrier discharge air plasma and zeolites synthesized at different Na2O/SiO2 ratios" @default.
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• W3201416458 doi "https://doi.org/10.1016/j.jiec.2021.09.003" @default.
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