Matches in SemOpenAlex for { <https://semopenalex.org/work/W3201440384> ?p ?o ?g. }
- W3201440384 abstract "Abstract Engineering the fate of supramolecular assemblies by heat treatment (i. e., using thermal preparative pathways) remains challenging and a largely ad hoc process. The rational design of such trajectories requires precise manipulation of the strength of molecularly encrypted interactions along an assembly path defined by changes in free energy as a function of temperature. Here, we use temperature‐triggered liquid–liquid phase separation of proteins to program the nano‐ and mesoscale assembly of a genetically encoded amphiphile – a post‐translationally lipidated protein – along user‐defined thermal trajectories. This molecularly defined pathway was used to funnel thermal energy into the system to direct building blocks to a previously inaccessible region of the energy landscape, and to synthesize two‐dimensional nanomaterials with sophisticated structures, such as braids and toroids. Because proteins’ phase boundaries and transition are programmable at the sequence‐level, our strategy opens new horizons to expand the structural hierarchy and functional landscape of protein‐based materials." @default.
- W3201440384 created "2021-09-27" @default.
- W3201440384 creator A5015877292 @default.
- W3201440384 creator A5018218412 @default.
- W3201440384 creator A5030864096 @default.
- W3201440384 creator A5077558876 @default.
- W3201440384 creator A5080141945 @default.
- W3201440384 creator A5080252826 @default.
- W3201440384 date "2021-10-22" @default.
- W3201440384 modified "2023-10-16" @default.
- W3201440384 title "Pathway‐Selection for Programmable Assembly of Genetically Encoded Amphiphiles by Thermal Processing" @default.
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