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- W3201499054 abstract "Aqueous sodium-ion batteries (ASIBs) are aspiring candidates for low environmental impact energy storage, especially when using organic electrodes. In this respect, perylene-3,4,9,10-tetracarboxylic dianhydride (PTCDA) is a promising anode active material, but it suffers from extensive dissolution in conventional aqueous electrolytes. As a remedy, we here present a novel aqueous electrolyte, which inhibits the PTCDA dissolution and enables their use as all-organic ASIB anodes with high capacity retention and Coulombic efficiencies. Furthermore, the electrolyte is based on two, hence hybrid, inexpensive and non-fluorinated Na/Mg-salts, it displays favourable physico-chemical properties and an electrochemical stability window >3 V without resorting to the extreme salt concentrations of water-in-salt electrolytes. Altogether, this paves the way for ASIBs with both relatively high energy densities, inexpensive total cell chemistries, long-term sustainability, and improved safety." @default.
- W3201499054 created "2021-09-27" @default.
- W3201499054 creator A5025870307 @default.
- W3201499054 creator A5025962179 @default.
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- W3201499054 date "2021-10-12" @default.
- W3201499054 modified "2023-10-16" @default.
- W3201499054 title "High‐Performant All‐Organic Aqueous Sodium‐Ion Batteries Enabled by PTCDA Electrodes and a Hybrid Na/Mg Electrolyte" @default.
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- W3201499054 doi "https://doi.org/10.1002/anie.202111620" @default.
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