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• W3201567461 abstract "Employing a ternary blend as absorber is an ingenious tactic to achieve broad spectral coverage in single-junction organic photovoltaics. The incorporation of a second acceptor with relatively lower electron affinity (EA) is important for attaining increased open-circuit voltage (VOC) of ternary devices. However, the common way in achieving a lower EA through tailoring the skeletons may affect the miscibility between acceptors, which inherently restrict the dependence of VOC on compositions. Herein, we developed a low-EA acceptor through side-chain engineering to ensure similarity with another ultranarrow-bandgap acceptor, enabling a good miscibility between the two species and formation of a vitrified solid solution over a large range of compositions. As a result, continuously increased VOC is realized, while the other parameters are less composition-sensitive. Besides, the vitrification facilitates intimate intermolecular interactions in ternary blends, suppressing thermally induced crystallization. Ultimately, increased photovoltaic efficiency and thermal stability are simultaneously achieved for the resulting ternary devices." @default.
• W3201567461 created "2021-09-27" @default.
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• W3201567461 date "2021-09-13" @default.
• W3201567461 modified "2023-10-14" @default.
• W3201567461 title "Formation of Vitrified Solid Solution Enables Simultaneously Efficient and Stable Organic Solar Cells" @default.
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• W3201567461 doi "https://doi.org/10.1021/acsenergylett.1c01576" @default.
• W3201567461 hasPublicationYear "2021" @default.
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