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- W3201628143 abstract "High-voltage spinel Li1+xNi0.5Mn1.5O4-xClx (0 ≤ x ≤ 0.04) cathode materials with different contents of Li+ and Cl− co-doping were obtained through a solid-state process. Scanning electron microscopy and transmission electron microscopy images indicate that pure LiNi0.5Mn1.5O4 (LNMO, space group Fd-3 m) particles possess an octahedral morphology, predominantly exhibiting {111} crystallographic planes. While the specimens with Li+ and Cl− co-doping display not only {111} crystal facets but also positive {100} and {110} facets (i.e. truncated octahedral shape) that could facilitate Li+ transport and stabilize the spinel structure. Compared to the pure LNMO, the Li+ and Cl− co-doped LNMO electrodes display superior electrochemical performances. For example, the Li1.03Ni0.5Mn1.5O3.97Cl0.03 exhibits the superior rate capability, with discharge capacities of 92.3 and 52.6 mA h g−1 at 7C and 10C, respectively, which are much higher than those of pure LNMO (54.2 and 7.8 mA h g−1 at 7C and 10C). An improved electrochemical properties of LNMO-Cl0.03 is attributable to its relatively larger portion of {100} and {110} facets, lower charge-transfer resistance and electrode polarization, and higher Li+ diffusion coefficient." @default.
- W3201628143 created "2021-09-27" @default.
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- W3201628143 date "2021-11-01" @default.
- W3201628143 modified "2023-10-18" @default.
- W3201628143 title "Li+ and Cl− co-doped LiNi0.5Mn1.5O4 cathode material with truncated octahedral shape and enhanced electrochemical performance for Li-ion batteries" @default.
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- W3201628143 doi "https://doi.org/10.1016/j.ssi.2021.115753" @default.
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